Authors
Mingjian Yuan, Li Na Quan, Riccardo Comin, Grant Walters, Randy Sabatini, Oleksandr Voznyy, Sjoerd Hoogland, Yongbiao Zhao, Eric M Beauregard, Pongsakorn Kanjanaboos, Zhenghong Lu, Dong Ha Kim, Edward H Sargent
Publication date
2016/10
Journal
Nature nanotechnology
Volume
11
Issue
10
Pages
872-877
Publisher
Nature Publishing Group UK
Description
Organometal halide perovskites exhibit large bulk crystal domain sizes, rare traps, excellent mobilities and carriers that are free at room temperature—properties that support their excellent performance in charge-separating devices. In devices that rely on the forward injection of electrons and holes, such as light-emitting diodes (LEDs), excellent mobilities contribute to the efficient capture of non-equilibrium charge carriers by rare non-radiative centres. Moreover, the lack of bound excitons weakens the competition of desired radiative (over undesired non-radiative) recombination. Here we report a perovskite mixed material comprising a series of differently quantum-size-tuned grains that funnels photoexcitations to the lowest-bandgap light-emitter in the mixture. The materials function as charge carrier concentrators, ensuring that radiative recombination successfully outcompetes trapping and hence non-radiative …
Total citations
20162017201820192020202120222023202412148280314340354294241130
Scholar articles
M Yuan, LN Quan, R Comin, G Walters, R Sabatini… - Nature nanotechnology, 2016
G Xing, B Wu, X Wu, M Li, B Du, Q Wei, J Guo… - Nat. Commun, 2017