Authors
Rafael M Santos, Davy François, Gilles Mertens, Jan Elsen, Tom Van Gerven
Publication date
2013/8/1
Journal
Applied Thermal Engineering
Volume
57
Issue
1-2
Pages
154-163
Publisher
Pergamon
Description
Several aspects of ultrasound-assisted mineral carbonation were investigated in this work. The objectives were to intensify the CO2 sequestration process to improve reaction kinetics and maximal conversion. Stainless steel slags, derived from the Argon Oxygen Decarburization (AOD) and Continuous Casting/Ladle Metallurgy (CC/LM) refining steps, were used for assessing the technical feasibility of this concept, as they are potential carbon sinks and can benefit from reduction in alkalinity (pH) by mineral carbonation. Ultrasound was applied by use of an ultrasound horn into the reaction slurry, where mineral carbonation reaction took place at 50 °C for up to 4 h; comparison was made to solely mechanically mixed process. It was found that sonication increases the reaction rate after the initial stage, and permits achieving higher carbonate conversion and lower pH. AOD slag conversion increased from 30% to 49 …
Total citations
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Scholar articles
RM Santos, D François, G Mertens, J Elsen… - Applied Thermal Engineering, 2013