Authors
Steve Albrecht, Michael Saliba, Juan Pablo Correa Baena, Felix Lang, Lukas Kegelmann, Mathias Mews, Ludmilla Steier, Antonio Abate, Jörg Rappich, Lars Korte, Rutger Schlatmann, Mohammad Khaja Nazeeruddin, Anders Hagfeldt, Michael Grätzel, Bernd Rech
Publication date
2016
Journal
Energy & Environmental Science
Volume
9
Issue
1
Pages
81-88
Publisher
Royal Society of Chemistry
Description
Tandem solar cells combining silicon and perovskite absorbers have the potential to outperform state-of-the-art high efficiency silicon single junction devices. However, the practical fabrication of monolithic silicon/perovskite tandem solar cells is challenging as material properties and processing requirements such as temperature restrict the device design. Here, we fabricate an 18% efficient monolithic tandem cell formed by a silicon heterojunction bottom- and a perovskite top-cell enabling a very high open circuit voltage of 1.78 V. The monolithic integration was realized via low temperature processing of the semitransparent perovskite sub-cell where an energetically aligned electron selective contact was fabricated by atomic layer deposition of tin oxide. The hole selective, transparent top contact was formed by a stack of the organic hole transport material spiro-OMeTAD, molybdenum oxide and sputtered indium …
Total citations
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