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This paper describes the results of an experimental and theoretical investigation into the mechanisms by which spume droplets are generated by high winds. The experiments were performed in a high-speed wind-wave flume at friction velocities between 0.8 and 1.5 m s ⁻¹ (corresponding to a 10-m wind speed of 18–33 m s ⁻¹ under field conditions). High-speed video of the air–water interface revealed that the main types of spray-generating phenomena near the interface are “bag breakup” (similar to fragmentation of droplets and jets in gaseous flows at moderate Weber numbers), breakage of liquid ligaments near the crests of breaking surface waves, and bursting of large submerged bubbles. Statistical analysis of these phenomena showed that at wind friction velocities exceeding 1.1 m s ⁻¹ (corresponding to a wind speed of approximately 22.5 m s ⁻¹ …