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Methods, systems, and media for relighting images using predicted deep reflectance fields are provided. In some embodiments, the method comprises: identifying a group of training samples, wherein each training sample includes (i) a group of one-light-at-a-time (OLAT) images that have each been captured when one light of a plurality of lights arranged on a lighting structure has been activated,(ii) a group of spherical color gradient images that have each been captured when the plurality of lights arranged on the lighting structure have been activated to each emit a particular color, and (iii) a lighting direction, wherein each image in the group of OLAT images and each of the spherical color gradient images are an image of a subject, and wherein the lighting direction indicates a relative orientation of a light to the subject; training a convolutional neural network using the group of training samples, wherein training …