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This paper assesses three key energy sustainability objectives: energy security improvement, climate change mitigation, and the reduction of air pollution and its human health impacts. We explain how the common practice of narrowly focusing on singular issues ignores potentially enormous synergies, highlighting the need for a paradigm shift toward more holistic policy approaches. Our analysis of a large ensemble of alternate energy-climate futures, developed using MESSAGE, an integrated assessment model, shows that stringent climate change policy offers a strategic entry point along the path to energy sustainability in several dimensions. Concerted decarbonization efforts can lead to improved air quality, thereby reducing energy-related health impacts worldwide: upwards of 2–32 million fewer disability-adjusted life years in 2030, depending on the aggressiveness of the air pollution policies …