Authors
Libin Wu, Hong Ren, Peng Wang, Jing Chen, Yunting Fang, Wei Hu, Lujie Ren, Junjun Deng, Yu Song, Jie Li, Yele Sun, Zifa Wang, Cong-Qiang Liu, Qi Ying, Pingqing Fu
Publication date
2019/6/24
Journal
Environmental Science & Technology Letters
Volume
6
Issue
7
Pages
389-395
Publisher
American Chemical Society
Description
This study investigates the concentrations and δ15N values of NH4+ in PM2.5 at three heights (8, 120, and 260 m) on a 325 m tower in urban Beijing. NH4+ concentrations were lower during the Parade Blue Period (August 20 to September 3, 2015) due to strict air pollution control and favorable meteorological conditions, while δ15N-NH4+ values were higher because the regional transport of agricultural sources (lower ratios of δ15N-NH4+) was less significant. Vertical profiles of NH4+ increased with height while δ15N-NH4+ decreased, indicating an enhanced contribution from regional transport at high altitudes. The results of the “MixSIAR” isotopic mixing model indicate that agricultural emission produces 47% of the ground-surface NH4+ and reaches 51–56% at high altitudes. Results from a source-oriented air quality model and the 2016 MEIC emission inventory suggest that non-agricultural NH3 emissions …
Total citations
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