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A spectral approach to building the exterior calculus in manifold learning problems is developed. The spectral approach is shown to converge to the true exterior calculus in the limit of large data. Simultaneously, the spectral approach decouples the memory requirements from the amount of data points and ambient space dimension. To achieve this, the exterior calculus is reformulated entirely in terms of the eigenvalues and eigenfunctions of the Laplacian operator on functions. The exterior derivatives of these eigenfunctions (and their wedge products) are shown to form a frame (a type of spanning set) for appropriate L² spaces of k‐forms, as well as higher‐order Sobolev spaces. Formulas are derived to express the Laplace‐de Rham operators on forms in terms of the eigenfunctions and eigenvalues of the Laplacian on functions. By representing the Laplace‐de Rham operators in this frame, spectral convergence …