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Numerical studies were performed to assess the quality and reliability of wall-modeled large eddy simulation (LES) for studying convective heat and mass transfer over bluff bodies at high Reynolds numbers (Re), with a focus on built structures in the atmospheric boundary layer. Detailed comparisons were made with both wind-tunnel experiments and field observations. The LES was shown to correctly capture the spatial patterns of the transfer coefficients around two-dimensional roughness ribs (with a discrepancy of about 20%) and the average Nusselt number (Nu) over a single wall mounted cube (with a discrepancy of about 25%) relative to wind tunnel measurements. However, the discrepancy in Re between the wind tunnel measurements and the real-world applications that the code aims to address influence the comparisons since Nu is a function of Re. Evaluations against field observations are therefore …