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High-precision time synchronization between satellites and ground stations plays the vital role in satellite navigation system. Laser time transfer (LTT) technology is widely recognized as the highest accuracy way to achieve time synchronization derived from satellite laser ranging (SLR) technology. Onboard LTT payload has been designed and developed by Shanghai Astronomical Observatory, and successfully applied to Chinese Beidou navigation satellites. By using the SLR system, with strictly controlling laser firing time and developing LTT data processing system on ground, the high precise onboard laser time transfer experiment has been first performed for satellite navigation system in the world. The clock difference and relative frequency difference between the ground hydrogen maser and space rubidium clocks have been obtained, with the precision of approximately 300ps and relative frequency stability …