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A three-dimensional model of the gold-rich Paleoproterozoic Ashanti Greenstone Belt has been built with a “hybrid” geological modeling method using Geomodeller and Gocad, then inverted using VPmg software. The model helps to identify the main regional-scale controls leading to abundant gold mineralization in the southeast of the belt by highlighting the lithological distribution and geometry of geological structures. The three-dimensional geological model shows that 85% of gold occurrences in the Ashanti Greenstone Belt are proximal to a specific tholeiitic metabasaltic horizon “BV1”. This result is noteworthy given that the relatively thin, 300 m thick, BV1 layer represents only 10%, by volume, of the modeled Sefwi Group stratigraphy. A map of distance between the topography and the BV1 layer is produced and identifies areas showing a high probability to host gold deposits in the southeast of the Ashanti Belt …