Authors
Zaiyao Fei, Bevin Huang, Paul Malinowski, Wenbo Wang, Tiancheng Song, Joshua Sanchez, Wang Yao, Di Xiao, Xiaoyang Zhu, Andrew F May, Weida Wu, David H Cobden, Jiun-Haw Chu, Xiaodong Xu
Publication date
2018/9
Journal
Nature materials
Volume
17
Issue
9
Pages
778-782
Publisher
Nature Publishing Group UK
Description
Discoveries of intrinsic two-dimensional (2D) ferromagnetism in van der Waals (vdW) crystals provide an interesting arena for studying fundamental 2D magnetism and devices that employ localized spins, , –. However, an exfoliable vdW material that exhibits intrinsic 2D itinerant magnetism remains elusive. Here we demonstrate that Fe3GeTe2 (FGT), an exfoliable vdW magnet, exhibits robust 2D ferromagnetism with strong perpendicular anisotropy when thinned down to a monolayer. Layer-number-dependent studies reveal a crossover from 3D to 2D Ising ferromagnetism for thicknesses less than 4 nm (five layers), accompanied by a fast drop of the Curie temperature (TC) from 207 K to 130 K in the monolayer. For FGT flakes thicker than ~15 nm, a distinct magnetic behaviour emerges in an intermediate temperature range, which we show is due to the formation of labyrinthine domain patterns. Our work …
Total citations
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