Authors
CS McNaughton, AD Clarke, S Freitag, VN Kapustin, Y Kondo, N Moteki, L Sahu, N Takegawa, JP Schwarz, JR Spackman, L Watts, G Diskin, J Podolske, JS Holloway, A Wisthaler, T Mikoviny, J De Gouw, C Warneke, J Jimenez, M Cubison, SG Howell, A Middlebrook, R Bahreini, BE Anderson, E Winstead, KL Thornhill, D Lack, J Cozic, CA Brock
Publication date
2011/8/1
Journal
Atmospheric Chemistry and Physics
Volume
11
Issue
15
Pages
7561-7582
Publisher
Copernicus GmbH
Description
In the spring of 2008 NASA and NOAA funded the ARCTAS and ARCPAC field campaigns as contributions to POLARCAT, a core IPY activity. During the campaigns the NASA DC-8, P-3B and NOAA WP-3D aircraft conducted over 160 h of in-situ sampling between 0.1 and 12 km throughout the Western Arctic north of 55° N (i.e. Alaska to Greenland). All aircraft were equipped with multiple wavelength measurements of aerosol optics, trace gas and aerosol chemistry measurements, as well as direct measurements of the aerosol size distributions and black carbon mass. Late April of 2008 proved to be exceptional in terms of Asian biomass burning emissions transported to the Western Arctic. Though these smoke plumes account for only 11–14 % of the samples within the Western Arctic domain, they account for 42–47 % of the total burden of black carbon. Dust was also commonly observed but only contributes to 4–12 % and 3–8 % of total light absorption at 470 and 530 nm wavelengths above 6 km. Below 6 km, light absorption by carbonaceous aerosol derived from urban/industrial and biomass burning emissions account for 97–99 % of total light absorption by aerosol. Stratifying the data to reduce the influence of dust allows us to determine mass absorption efficiencies for black carbon of 11.2±0.8, 9.5±0.6 and 7.4±0.7 m2 g−1 at 470, 530 and 660 nm wavelengths. These estimates are consistent with 35–80 % enhancements in 530 nm absorption due to clear or slightly absorbing coatings of pure black carbon particulate. Assuming a 1/λ wavelength dependence for BC absorption, and assuming that refractory aerosol (420 °C, τ = 0.1 s) in low …
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