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We investigated relations among strengths of character in 881 students from Croatian universities. We also examined links between strengths and various well-being indices. Our conceptualization was based on the Values in Action classification system with 24 strengths organized within six superordinate virtues (Peterson & Seligman, 2004). A factor analysis led to a four-factor solution; factors were defined as Interpersonal Strengths, Fortitude, Vitality, and Cautiousness. Of these factors, Vitality (with zest, hope, curiosity, and humor as indicators) emerged as the most relevant to well-being. When examining individual strengths, zest, curiosity, gratitude, and optimism/hope emerged with the strongest associations with elevated life satisfaction, subjective vitality, satisfaction of autonomy, relatedness, and competence needs, and a pleasurable, engaging, and meaningful existence. Results have implications for …