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To enhance the energy security and promote energy diversity, biomass sources of energy are viable resources worldwide. Bioenergy is an organic source of power derived from various feedstock including fuel wood, energy crops, solid wastes, and residues of plants. This book chapter explores the use of biomass in Africa and the technical and economic potential of these resources for energy supply in the continent. Findings of literature revealed that the potential of biomass is high in Africa due to availability of land, its preference due to limited electricity supply and the exorbitant nature of fossil fuels, the assorted variety of energy crops suitable for growth in the continent and the green nature associated with the resource. The chapter also established that bioenergy is renewable and not carbon neutral. As such, accurate computation of its resultant greenhouse gas emissions based on their sequestration and emission rates is strongly advised to optimize biomass for energy utility and sustainability compared to conventional energy sources.