Authors
Vincent Mauchamp, Matthieu Bugnet, Edson P Bellido, Gianluigi A Botton, Philippe Moreau, Damien Magne, Michael Naguib, Thierry Cabioc'h, Michel W Barsoum
Publication date
2014/6/15
Journal
Physical Review B
Volume
89
Issue
23
Pages
235428
Publisher
American Physical Society
Description
The dielectric response of two-dimensional (2D) stacked sheets was investigated by high-resolution transmission electron energy-loss spectroscopy and ab initio calculations in the 0.2–30-eV energy range. Intense surface plasmons (SPs), evidenced at the nanometer scale at energies as low as 0.3 eV, are shown to be the dominant screening process up to at least 45-nm-thick stacks. This domination results from a combination of efficient free-electron dynamics, begrenzungs effect, and reduced interband damping. It is shown that, in principle, the SPs energies can be tuned in the mid-infrared, from 0.2 to 0.7 eV, by controlling the sheets' functionalization and/or thickness. This point evidences a new attribute of this new class of 2D materials.
Total citations
201420152016201720182019202020212022202320242106811142330291912