Authors
Jan M Winkler, Freddy T Rabouw, Aurelio A Rossinelli, Sriharsha V Jayanti, Kevin M McPeak, David K Kim, Boris Le Feber, Ferry Prins, David J Norris
Publication date
2018/12/5
Journal
Nano letters
Volume
19
Issue
1
Pages
108-115
Publisher
American Chemical Society
Description
Exciton polaritons are hybrid light–matter quasiparticles that can serve as coherent light sources. Motivated by applications, room-temperature realization of polaritons requires narrow, excitonic transitions with large transition dipoles. Such transitions must then be strongly coupled to an electromagnetic mode confined in a small volume. While much work has explored polaritons in organic materials, semiconductor nanocrystals present an alternative excitonic system with enhanced photostability and spectral tunability. In particular, quasi-two-dimensional nanocrystals known as nanoplatelets (NPLs) exhibit intense, spectrally narrow excitonic transitions useful for polariton formation. Here, we place CdSe NPLs on silver hole arrays to demonstrate exciton–plasmon polaritons at room temperature. Angle-resolved reflection spectra reveal Rabi splittings up to 149 meV for the polariton states. We observe bright, polarized …
Total citations
2019202020212022202320243109686
Scholar articles