Authors
Alma Hodzic, Sasha Madronich, B Bohn, S Massie, L Menut, Christine Wiedinmyer
Publication date
2007/8/2
Journal
Atmospheric Chemistry and Physics
Volume
7
Issue
15
Pages
4043-4064
Publisher
Copernicus Publications
Description
The present study investigates effects of wildfire emissions on air quality in Europe during an intense fire season that occurred in summer 2003. A meso-scale chemistry transport model CHIMERE is used, together with ground based and satellite aerosol optical measurements, to assess the dispersion of fire emissions and to quantify the associated radiative effects. The model has been improved to take into account a MODIS-derived daily smoke emission inventory as well as the injection altitude of smoke particles. The simulated aerosol optical properties are put into a radiative transfer model to estimate (off-line) the effects of smoke particles on photolysis rates and atmospheric radiative forcing. We have found that the simulated wildfires generated comparable amounts of primary aerosol pollutants (130 kTons of PM2.5, fine particles) to anthropogenic sources during August 2003, and caused significant changes in aerosol optical properties not only close to the fire source regions, but also over a large part of Europe as a result of the long-range transport of the smoke. Including these emissions into the model significantly improved its performance in simulating observed aerosol concentrations and optical properties. Quantitative comparison with MODIS and POLDER data during the major fire event (3–8 August 2003) showed the ability of the model to reproduce high aerosol optical thickness (AOT) over Northern Europe caused by the advection of the smoke plume from the Portugal source region. Although there was a fairly good spatial agreement with satellite data (correlation coefficients ranging from 0.4 to 0.9), the temporal variability of AOT …
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