Authors
Joel Yuen-Zhou, David G Tempel, César A Rodríguez-Rosario, Alán Aspuru-Guzik
Publication date
2010/1/29
Journal
Physical review letters
Volume
104
Issue
4
Pages
043001
Publisher
American Physical Society
Description
We extend the Runge-Gross theorem for a very general class of open quantum systems under weak assumptions about the nature of the bath and its coupling to the system. We show that for Kohn-Sham (KS) time-dependent density functional theory, it is possible to rigorously include the effects of the environment within a bath functional in the KS potential. A Markovian bath functional inspired by the theory of nonlinear Schrödinger equations is suggested, which can be readily implemented in currently existing real-time codes. Finally, calculations on a helium model system are presented.
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