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High-precision time synchronization for remote clocks plays an important role in fundamental science^{, –} and real-life applications^,. However, current time synchronization techniques^, have been shown to be vulnerable to sophisticated adversaries. There is a compelling need for fundamentally new methods to distribute high-precision time information securely. Here, we propose a satellite-based quantum-secure time transfer (QSTT) scheme based on two-way quantum key distribution in free space and experimentally verify the key technologies of the scheme via the Micius quantum satellite. In QSTT, a quantum signal (for example, a single photon) is used as the carrier for both the time transfer and the secret-key generation, offering quantum-enhanced security for transferring the time signal and time information. We perform a satellite-to-ground time synchronization using single-photon-level signals and achieve a …