Authors
Peter B Kelemen, Noah McQueen, Jennifer Wilcox, Phil Renforth, Greg Dipple, Amelia Paukert Vankeuren
Publication date
2020/9/20
Source
Chemical Geology
Volume
550
Pages
119628
Publisher
Elsevier
Description
Carbon Dioxide removal from air (CDR) combined with permanent solid storage can be accomplished via carbon mineralization in ultramafic rocks in at least four ways:
1. Surficial CDR: CO2-bearing air and surface waters are reacted with crushed and or ground mine tailings, alkaline industrial wastes, or sedimentary formations rich in reactive rock fragments, all with a high proportion of reactive surface area. This can be implemented at a low cost, but most proposed methods have a very large area footprint at the gigatonne scale. The area requirement can be greatly reduced by calcining (heating to produce pure CO2 for permanent storage or use) followed by recycling of MgO, CaO, Na2O, … Such looping methods have predicted costs that are as low or lower than for direct air capture with synthetic sorbents or solvents (DACSS), and a similar area footprint.
2. In situ CDR: CO2-bearing surface waters are circulated …
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