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There has been a recent demand for the development of luminescent materials for visualizations of latent fingerprints (LFPs) for achieving enhanced security. Also recently, there has been a new research trend in the development of 2D materials from non-layered semiconductors with strong luminescence properties in the visible region. The conventional growth process of luminescent materials limits their capacity of tuning the structure and light emission efficiency. However, multi-atom doping provides an additional degree of freedom to tune the basic morphologies and optical properties of luminescent semiconductors by controlling the defect levels. Here, by using a simple chemical technique, multi-atom (Cu and Mn) doped rarely reported 2D nanosheets of zinc sulphide (ZnS) have been grown. Thus, a stable high fluorescence efficiency of ∼62% in the visible region has been realized for the visualization of LFPs …