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The development of smart infrastructures is a political act that intersects, in powerful ways, with ongoing decolonial struggles across the uneven landscapes of the postcolonial world. This paper develops a grounded, relational approach to the critical geographies of smart development that starts from place‐based relations of power to investigate how specific postcolonial dynamics inflect the global articulation of smart development. Drawing on the work of Gillian Hart, our approach situates the development of smart infrastructures within longer, contested histories of geopolitical intervention and capitalist transformation and foregrounds ongoing land, labour and livelihood struggles that transect the urban–rural divide. Using critical ethnography and relational comparison in South East Asia and the Middle East, we show how Myanmar's smart farms and Jordan's smart grid were built and selectively adapted or refused …