Authors
Young Chul Jun, Ragip Pala, Mark L Brongersma
Publication date
2010/4/29
Journal
The Journal of Physical Chemistry C
Volume
114
Issue
16
Pages
7269-7273
Publisher
American Chemical Society
Description
A metal−dielectric−metal (MDM) waveguide with a nanoscale gap supports highly confined surface plasmon−polariton modes, termed gap plasmons. The spontaneous emission of an emitter placed in such a metal nanogap is expected to be strongly modified due to coupling to gap plasmons. We investigate the light emission properties of semiconductor quantum dots (QD) in a metal nanoslit, which is a truncated MDM waveguide. More specifically, we measure both the lifetime and the state of polarization of the out-coupled QD emission from a metal nanoslit. We observe clear lifetime and polarization changes of QD emission. As the slit width gets smaller, the QD exciton lifetime gradually decreases, and its emission becomes polarized normal to the slit, as expected for gap plasmon coupled light emission. We also find that the polarization of the collected QD emission is flipped (i.e., becomes parallel to a slit) when …
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