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Many applications proposed for functional nanofibers require their assembly into a monolithic cellular structure. The ability to maintain structural integrity upon large deformation is essential to ensure a macroscopic cellular material that functions reliably. However, it remains a great challenge to achieve high elasticity in three-dimensional (3D) nanofibrous networks. Here, we report a strategy to create fibrous, isotropically bonded elastic reconstructed (FIBER) aerogels with a hierarchical cellular structure and superelasticity by combining electrospun nanofibers and the freeze-shaping technique. Our approach allows the intrinsically lamellar deposited electrospun nanofibers to assemble into elastic bulk aerogels with tunable porous structure and wettability on a large scale. The resulting FIBER aerogels exhibit the integrated properties of ultralow density (<30 mg cm^–3), rapid recovery from 80% compression strain …