Authors
Rafael M Santos, Jens Van Bouwel, Ellen Vandevelde, Gilles Mertens, Jan Elsen, Tom Van Gerven
Publication date
2013/9/1
Journal
International Journal of Greenhouse Gas Control
Volume
17
Pages
32-45
Publisher
Elsevier
Description
This work explores the mineral carbonation of stainless steel slags in search for a technically and economically feasible treatment solution that steers these waste residues away from costly disposal in landfills and into valuable applications. Argon Oxygen Decarburization (AOD) and Continuous Casting (CC) slags prove ideal for mineral carbonation as their powdery morphology forgoes the need for milling and provides sufficient surface area for high reactivity towards direct aqueous carbonation. Experiments were undertaken using two methodologies: unpressurized thin-film carbonation, and pressurized slurry carbonation. The influence of process parameters (temperature, CO2 partial pressure, time, and solids loading) on the slag carbonation conversion are investigated, seeking the optimal conditions that maximize the potential of the slags as carbon sinks. It was found that CC slag carbonates more extensively …
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