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We propose a novel structured analysis–synthesis dictionary pair learning method for efficient representation and image classification, referred to as relaxed block-diagonal dictionary pair learning with a locality constraint (RBD-DPL). RBD-DPL aims to learn relaxed block-diagonal representations of the input data to enhance the discriminability of both analysis and synthesis dictionaries by dynamically optimizing the block-diagonal components of representation, while the off-block-diagonal counterparts are set to zero. In this way, the learned synthesis subdictionary is allowed to be more flexible in reconstructing the samples from the same class, and the analysis dictionary effectively transforms the original samples into a relaxed coefficient subspace, which is closely associated with the label information. Besides, we incorporate a locality-constraint term as a complement of the relaxation learning to enhance the locality …