Authors
Ioanna Dimitriou, Pelayo García-Gutiérrez, Rachael H Elder, Rosa M Cuéllar-Franca, Adisa Azapagic, Ray WK Allen
Publication date
2015
Journal
Energy & Environmental Science
Volume
8
Issue
6
Pages
1775-1789
Publisher
Royal Society of Chemistry
Description
Utilising CO2 as a feedstock for chemicals and fuels could help mitigate climate change and reduce dependence on fossil fuels. For this reason, there is an increasing world-wide interest in carbon capture and utilisation (CCU). As part of a broader project to identify key technical advances required for sustainable CCU, this work considers different process designs, each at a high level of technology readiness and suitable for large-scale conversion of CO2 into liquid hydrocarbon fuels, using biogas from sewage sludge as a source of CO2. The main objective of the paper is to estimate fuel production yields and costs of different CCU process configurations in order to establish whether the production of hydrocarbon fuels from commercially proven technologies is economically viable. Four process concepts are examined, developed and modelled using the process simulation software Aspen Plus® to determine raw …
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