Authors
G Trinkunas, JL Herek, T Polivka, V Sundström, T Pullerits
Publication date
2001/4/30
Journal
Physical Review Letters
Volume
86
Issue
18
Pages
4167
Publisher
American Physical Society
Description
Singlet-singlet annihilation is used to study exciton delocalization in the light harvesting antenna complex LH2 (B800-B850) from the photosynthetic purple bacterium Rhodobacter sphaeroides. The characteristic femtosecond decay constants of the high intensity isotropic and the low intensity anisotropy kinetics of the B850 ring are related to the hopping time τ h and the coherence length N coh of the exciton. Our analysis yields N coh= 2.8±0.4 and τ h= 0.27±0.05 ps. This approach can be seen as an extension to the concept of the spectroscopic ruler.
Total citations
Scholar articles
G Trinkunas, JL Herek, T Polivka, V Sundström… - Physical Review Letters, 2001