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The control on megathrust earthquake generation exerted by deeper subduction processes remains poorly understood and still insufficiently documented. Here, we use the 2003-2014 space-time variations of the Earth's gravity gradients derived from the GRACE geoids in order to probe aseismic mass variations at depth and their possible interactions with intraplate seismicity along the Chilean margin. We work with three different datasets of GRACE geoid models over a large region surrounding the rupture zone of the Mw 8.8 2010 Maule earthquake. In order to separate signals associated with mass sources of differents sizes, shapes or orientations, we reconstruct each month the Earth's gravity gradients at different spatial scales from these geoid models. Our analysis emphasizes a highly anomalous, large-amplitude gravity gradients signal that appears three months prior to the earthquake North of the epicentral …