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Subduction zones megathrust faults constitute a considerable hazard as they produce most of the world's largest earthquakes. However, the role in megathrust earthquake generation exerted by deeper subduction processes remains poorly understood. Here, we analyze the 2003–2014 space-time variations of the Earth's gravity gradients derived from three datasets of GRACE geoid models over a large region surrounding the rupture zone of the Mw 8.8 Maule earthquake. In all these datasets, our analysis reveals a large-amplitude gravity gradient signal, progressively increasing in the three months before the earthquake, North of the epicentral area. We show that such signals are equivalent to a 60 km 3 water storage decrease over 2 months and cannot be explained by hydrological sources nor artefacts, but rather find origin from mass redistributions within the solid Earth on the continental side of the subduction …