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We investigate model theoretic characterisations of the expressive power of modal logics in terms of bisimulation invariance. The paradigmatic result of this kind is van Benthem’s theorem, which says that a first-order formula is invariant under bisimulation if, and only if, it is equivalent to a formula of basic modal logic. The present investigation primarily concerns ramifications for specific classes of structures. We study in particular model classes defined through conditions on the underlying frames, with a focus on frame classes that play a major role in modal correspondence theory and often correspond to typical application domains of modal logics. Classical model theoretic arguments do not apply to many of the most interesting classes–for instance, rooted frames, finite rooted frames, finite transitive frames, well-founded transitive frames, finite equivalence frames–as these are not elementary. Instead we develop …